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Detecting mid-infrared light by molecular frequency upconversion in dual-wavelength nanoantennas

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Peer-reviewed

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Article

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Authors

Zheng, Xuezhi 
Koczor-Benda, Zsuzsanna  ORCID logo  https://orcid.org/0000-0002-6714-0337

Abstract

jats:titleOptomechanical upconversion</jats:title> jats:p Molecules have rich signatures in their spectra at infrared wavelengths and are typically accessed with dedicated spectroscopic instrumentation. Chen jats:italicet al</jats:italic> . and Xomalis jats:italicet al</jats:italic> . report optomechanical frequency upconversion from the mid-infrared to the visible domain using molecular vibrations coupled to a plasmonic nanocavity at ambient conditions (see the Perspective by Gordon). Using different nanoantenna designs, one with a nanoparticle-on-resonator and the other with nanoparticle-in-groove, both approaches show the ability to upconvert the mid-infrared vibrations of the molecules in the nanocavity to visible light wavelengths. The effect could be used to simplify infrared spectroscopy, possibly with single-molecule sensitivity. —ISO </jats:p>

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Science

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Journal ISSN

0036-8075
1095-9203

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Publisher

American Association for the Advancement of Science (AAAS)
Sponsorship
Engineering and Physical Sciences Research Council (EP/L027151/1)
European Commission Horizon 2020 (H2020) Future and Emerging Technologies (FET) (829067)
European Commission Horizon 2020 (H2020) Research Infrastructures (RI) (861950)
European Commission Horizon 2020 (H2020) ERC (883703)
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