Content Source Figure 1 HOMO LUMO levels UPS + PDS (Figure--S2-1.zip + Figure--S2-2.zip) Figure 2 TA maps Figure--2.zip Figure 3 Charge generation times Figure--3--1-1.zip & Figure--3--1-1.zip Figure 4 Pump-Push-Photocurrent Figure--4--S5-1--S5-2.zip Figure 5 Scheme CS / CT - Figure S1.1 UV-Vis Figure--S1-1--S1-2.zip Figure S1.2 UV-Vis + CT emission Figure--S1-1--S1-2.zip Figure S2.1 UPS measurements Figure--S2-1.zip Figure S2.2 PDS measurements Figure--S2-2.zip Figure S2.3 HOMO LUMO levels Literature Figure S3 SAXS / WAXS Measurements Figure--S3.zip Figure S4.1 Charge generation times Figure--3--1-1.zip & Figure--3--1-1.zip Figure S4.2 Stimulated emission kinetics Figure--3--1-1.zip & Figure--3--1-1.zip Figure S4.3 TA kinetics (comparison) Figure--S4-3--S4-4.zip Figure S4.4 TA kinetics (fluence series) Figure--S4-3--S4-4.zip Figure S5.1 Pump-Push-Photocurrent (vs. d(LUMO)) Figure--4--S5-1--S5-2.zip Figure S5.2 Pump-Push-Photocurrent (temperature) Figure--4--S5-1--S5-2.zip File types: .ddt Transient Absorption data, ASCII file 1st Column: Wavelength (nm) 2nd Column: Time (ps or fs) - indicated by extra file in folder .tif SAXS/WAXS Data Software needed to open: Scatterbrain (http://www.synchrotron.org.au/aussyncbeamlines/saxswaxs/software-saxswaxs , opened 10-Aug-2016) .dat SAXS/WAXS Data, ASCII file .txt UPS, PDS, Pump-Push-Photocurrent, Absorption, Photoluminescence data: ASCII files