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dc.contributor.authorZhang, Dongdaen
dc.contributor.authorVassiliadis, Vassilien
dc.date.accessioned2015-06-25T13:33:48Z
dc.date.available2015-06-25T13:33:48Z
dc.date.issued2015-10-06en
dc.identifier.citationIndustrial and Engineering Chemistry Research 2015, 54(3): 10593–10605. doi: 10.1021/acs.iecr.5b02034en
dc.identifier.issn0888-5885
dc.identifier.urihttps://www.repository.cam.ac.uk/handle/1810/248717
dc.description.abstractThis paper presents a novel structured dynamic model to simulate the metabolic reaction network of green algae hydrogen production from aerobic condition to anaerobic condition, which has not been addressed in the open literature to this date. An efficient parameter estimation methodology is proposed to avoid the difficulty of measuring essential kinetic parameters from experiments. The accuracy of the model is verified by comparison to published experimental results. The current model finds that the starch generation pathway mainly competes with hydrogen production pathway, as its activity is enhanced by the cyclic electron flow pathway. From the dynamic sensitivity analysis, it is concluded that the most effective solution to enhance hydrogen production is to seek the optimal sulphur concentration in the culture, rather than to modify the activity of specific enzymes. The current work also denies the previous hypothesis that the diffusion of small proteins in the metabolic network inhibits hydrogen production.
dc.languageEnglishen
dc.language.isoenen
dc.publisherAmerican Chemical Society
dc.titleChlamydomonas reinhardtii Metabolic Pathway Analysis for Biohydrogen Production under Non-Steady State Operationen
dc.typeArticle
dc.description.versionThis is the accepted manuscript. The final version is available from ACS via http://dx.doi.org/10.1021/acs.iecr.5b02034en
prism.endingPage10605
prism.publicationDate2015en
prism.publicationNameIndustrial and Engineering Chemistry Researchen
prism.startingPage10593
prism.volume54en
rioxxterms.versionofrecord10.1021/acs.iecr.5b02034en
rioxxterms.licenseref.urihttp://www.rioxx.net/licenses/all-rights-reserveden
rioxxterms.licenseref.startdate2015-10-06en
dc.contributor.orcidVassiliadis, Vassili [0000-0002-5415-7551]
dc.identifier.eissn1520-5045
rioxxterms.typeJournal Article/Reviewen
rioxxterms.freetoread.startdate2016-10-06


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