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Capillary-Force-Assisted Optical Tuning of Coupled Plasmons.


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Authors

Ding, Tao 
Mertens, Jan 
Sigle, Daniel O 
Baumberg, Jeremy J 

Abstract

An ultrathin (few nanometer) polymer spacer layer is softened by local optical heating and restructured by strong capillary forces, which increase the gap between the plasmonic metal components. This results in a continuous blue-shift of the coupled plasmon from near infrared to visible with a tuning range of >150 nm that can be tightly controlled by adjusting either irradiation time or power.

Description

Keywords

gold, nanogaps, plasmon resonance, polymer spacer layers, spectra, Gold, Lasers, Metal Nanoparticles, Microscopy, Electron, Scanning, Polymers

Journal Title

Adv Mater

Conference Name

Journal ISSN

0935-9648
1521-4095

Volume Title

27

Publisher

Wiley
Sponsorship
Engineering and Physical Sciences Research Council (EP/G060649/1)
Engineering and Physical Sciences Research Council (EP/L027151/1)
European Research Council (320503)
Engineering and Physical Sciences Research Council (EP/K028510/1)
This work was supported by UK EPSRC grants EP/G060649/1, EP/L027151/1, and ERC grant LINASS 320503