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Large-scale quantum-emitter arrays in atomically thin semiconductors.

Published version
Peer-reviewed

Type

Article

Change log

Authors

Palacios-Berraquero, Carmen 
Kara, Dhiren M 
Montblanch, Alejandro R-P 
Barbone, Matteo 
Latawiec, Pawel 

Abstract

Quantum light emitters have been observed in atomically thin layers of transition metal dichalcogenides. However, they are found at random locations within the host material and usually in low densities, hindering experiments aiming to investigate this new class of emitters. Here, we create deterministic arrays of hundreds of quantum emitters in tungsten diselenide and tungsten disulphide monolayers, emitting across a range of wavelengths in the visible spectrum (610-680 nm and 740-820 nm), with a greater spectral stability than their randomly occurring counterparts. This is achieved by depositing monolayers onto silica substrates nanopatterned with arrays of 150-nm-diameter pillars ranging from 60 to 190 nm in height. The nanopillars create localized deformations in the material resulting in the quantum confinement of excitons. Our method may enable the placement of emitters in photonic structures such as optical waveguides in a scalable way, where precise and accurate positioning is paramount.

Description

Keywords

cond-mat.mes-hall, cond-mat.mes-hall, quant-ph

Journal Title

Nat Commun

Conference Name

Journal ISSN

2041-1723
2041-1723

Volume Title

8

Publisher

Springer Science and Business Media LLC
Sponsorship
Engineering and Physical Sciences Research Council (EP/K01711X/1)
Engineering and Physical Sciences Research Council (EP/K017144/1)
Engineering and Physical Sciences Research Council (EP/L016087/1)
EPSRC (via University of Manchester) (R119256)
Engineering and Physical Sciences Research Council (EP/M507799/1)
Engineering and Physical Sciences Research Council (EP/M013243/1)
Engineering and Physical Sciences Research Council (EP/G037221/1)
European Commission Horizon 2020 (H2020) Marie Sk?odowska-Curie actions (676108)