Field effect transistors and phototransistors based upon p-type solution-processed PbS nanowires.

Authors
Giraud, Paul 
Pak, Sangyeon 
Sohn, Jung Inn 
Morris, Stephen 

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Abstract

We demonstrate the fabrication of solution processed highly crystalline p-type PbS nanowires via the oriented attachment of nanoparticles. The analysis of single nanowire field effect transistor (FET) devices revealed a hole conduction behaviour with average mobilities greater than 30 cm2 V-1 s-1, which is an order of magnitude higher than that reported to date for p-type PbS colloidal nanowires. We have investigated the response of the FETs to near-infrared light excitation and show herein that the nanowires exhibited gate-dependent photo-conductivities, enabling us to tune the device performances. The responsivity was found to be greater than 104 A W-1 together with a detectivity of 1013 Jones, which benefits from a photogating effect occurring at negative gate voltages. These encouraging detection parameters are accompanied by relatively short switching times of 15 ms at positive gate voltages, resulting from a combination of the standard photoconduction and the high crystallinity of the nanowires. Collectively, these results indicate that solution-processed PbS nanowires are promising nanomaterials for infrared photodetectors as well as p-type nanowire FETs.

Publication Date
2018-02-16
Online Publication Date
2018-01-11
Acceptance Date
Keywords
nanowire FET, PbS, colloidal synthesis, p-type nanowires, phototransistor, photodetector
Journal Title
Nanotechnology
Journal ISSN
0957-4484
1361-6528
Volume Title
29
Publisher
IOP Publishing
Sponsorship
European Research Council (340538)
European Commission Horizon 2020 (H2020) Research Infrastructures (RI) (685758)