Linear and Nonlinear Spectroscopy by a Common-Path Birefringent Interferometer

Authors
Preda, F 
Oriana, A 
Rehault, J 
Lombardi, L 
Ferrari, AC 

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Type
Article
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Abstract

© 1995-2012 IEEE. We introduce a passive common-path interferometer to replace Michelson interferometers in the Fourier-Transform spectroscopy. Our device exploits birefringence to introduce a highly accurate delay between two orthogonal polarization components by continuously varying the material thickness. Due to its inherent delay stability and reproducibility, it can be used even for short wavelengths (down to ∼200 nm) without the need for any active control or position tracking. We first demonstrate its performances in linear spectroscopy, by implementing a spectrometer and a spectrophotometer. We then extend its use to nonlinear spectroscopy and, in combination with lock-in detection at MHz modulation frequencies, illustrate its application to pump-probe spectroscopy with high sensitivity (ΔT/T < 3·10 -6 in 1-s integration time) and broad spectral coverage ( > 500 nm) and to broadband stimulated Raman scattering microscopy in the CH stretching region.

Publication Date
2017-05-01
Online Publication Date
2016-12-05
Acceptance Date
2017-05-01
Keywords
Fourier-transform spectroscopy, ultrafast optics, coherent Raman scattering, pump-probe
Journal Title
IEEE Journal on Selected Topics in Quantum Electronics
Journal ISSN
1077-260X
1558-4542
Volume Title
23
Publisher
IEEE
Sponsorship
Engineering and Physical Sciences Research Council (EP/L016087/1)
EPSRC (via University of Manchester) (R119256)
European Research Council (319277)
Engineering and Physical Sciences Research Council (EP/K01711X/1)
Engineering and Physical Sciences Research Council (EP/K017144/1)
Engineering and Physical Sciences Research Council (EP/M507799/1)
European Commission Horizon 2020 (H2020) Future and Emerging Technologies (FET) (696656)