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Climate change modulates the stratospheric volcanic sulfate aerosol lifecycle and radiative forcing from tropical eruptions

Published version
Peer-reviewed

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Authors

Aubry, Thomas J. 
Staunton-Sykes, John  ORCID logo  https://orcid.org/0000-0001-9421-6897
Marshall, Lauren R.  ORCID logo  https://orcid.org/0000-0003-1471-9481
Abraham, Nathan Luke  ORCID logo  https://orcid.org/0000-0003-3750-3544

Abstract

Abstract: Explosive volcanic eruptions affect climate, but how climate change affects the stratospheric volcanic sulfate aerosol lifecycle and radiative forcing remains unexplored. We combine an eruptive column model with an aerosol-climate model to show that the stratospheric aerosol optical depth perturbation from frequent moderate-magnitude tropical eruptions (e.g. Nabro 2011) will be reduced by 75% in a high-end warming scenario compared to today, a consequence of future tropopause height rise and unchanged eruptive column height. In contrast, global-mean radiative forcing, stratospheric warming and surface cooling from infrequent large-magnitude tropical eruptions (e.g. Mt. Pinatubo 1991) will be exacerbated by 30%, 52 and 15% in the future, respectively. These changes are driven by an aerosol size decrease, mainly caused by the acceleration of the Brewer-Dobson circulation, and an increase in eruptive column height. Quantifying changes in both eruptive column dynamics and aerosol lifecycle is therefore key to assessing the climate response to future eruptions.

Description

Keywords

Article, /704/106/35, /704/106/35/824, /704/106/694, /704/2151/598, article

Journal Title

Nature Communications

Conference Name

Journal ISSN

2041-1723

Volume Title

12

Publisher

Nature Publishing Group UK
Sponsorship
RCUK | Natural Environment Research Council (NERC) (NE/T006897/1, NE/S000887/1, NE/T006897/1)
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