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dc.contributor.authorZhao, Run
dc.contributor.authorYang, Chao
dc.contributor.authorWang, Hongguang
dc.contributor.authorJiang, Kai
dc.contributor.authorWu, Hua
dc.contributor.authorShen, Shipeng
dc.contributor.authorWang, Le
dc.contributor.authorSun, Young
dc.contributor.authorJin, Kuijuan
dc.contributor.authorGao, Ju
dc.contributor.authorChen, Li
dc.contributor.authorWang, Haiyan
dc.contributor.authorMacManus-Driscoll, Judith L
dc.contributor.authorvan Aken, Peter A
dc.contributor.authorHong, Jiawang
dc.contributor.authorLi, Weiwei
dc.contributor.authorYang, Hao
dc.date.accessioned2022-06-07T08:15:35Z
dc.date.available2022-06-07T08:15:35Z
dc.date.issued2022-05-02
dc.identifier.issn2041-1723
dc.identifier.other35501352
dc.identifier.otherPMC9061821
dc.identifier.urihttps://www.repository.cam.ac.uk/handle/1810/337809
dc.description.abstractNegative pressure has emerged as a powerful tool to tailor the physical properties of functional materials. However, a negative pressure control of spin-phonon coupling for engineering magnetism and multiferroicity has not been explored to date. Here, using uniform three-dimensional strain-induced negative pressure in nanocomposite films of (EuTiO3)0.5:(MgO)0.5, we demonstrate an emergent multiferroicity with magnetodielectric coupling in EuTiO3, matching exactly with density functional theory calculations. Density functional theory calculations are further used to explore the underlying physics of antiferromagnetic-paraelectric to ferromagnetic-ferroelectric phase transitions, the spin-phonon coupling, and its correlation with negative pressures. The observation of magnetodielectric coupling in the EuTiO3 reveals that an enhanced spin-phonon coupling originates from a negative pressure induced by uniform three-dimensional strain. Our work provides a route to creating multiferroicity and magnetoelectric coupling in single-phase oxides using a negative pressure approach.
dc.languageeng
dc.publisherSpringer Science and Business Media LLC
dc.rightsAttribution 4.0 International
dc.rights.urihttps://creativecommons.org/licenses/by/4.0/
dc.sourcenlmid: 101528555
dc.sourceessn: 2041-1723
dc.titleEmergent multiferroism with magnetodielectric coupling in EuTiO3 created by a negative pressure control of strong spin-phonon coupling.
dc.typeArticle
dc.date.updated2022-06-07T08:15:35Z
prism.issueIdentifier1
prism.publicationNameNat Commun
prism.volume13
dc.identifier.doi10.17863/CAM.85218
dcterms.dateAccepted2022-04-15
rioxxterms.versionofrecord10.1038/s41467-022-30074-4
rioxxterms.versionVoR
rioxxterms.licenseref.urihttps://creativecommons.org/licenses/by/4.0/
dc.contributor.orcidYang, Chao [0000-0002-8630-590X]
dc.contributor.orcidWang, Hongguang [0000-0001-8552-2323]
dc.contributor.orcidJiang, Kai [0000-0002-5117-6941]
dc.contributor.orcidJin, Kuijuan [0000-0002-0047-4375]
dc.contributor.orcidWang, Haiyan [0000-0002-7397-1209]
dc.contributor.orcidMacManus-Driscoll, Judith L [0000-0003-4987-6620]
dc.contributor.orcidvan Aken, Peter A [0000-0003-1890-1256]
dc.contributor.orcidHong, Jiawang [0000-0002-9915-8072]
dc.contributor.orcidLi, Weiwei [0000-0001-5781-5401]
dc.contributor.orcidYang, Hao [0000-0002-9055-7165]
dc.identifier.eissn2041-1723
cam.issuedOnline2022-05-02


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Attribution 4.0 International
Except where otherwise noted, this item's licence is described as Attribution 4.0 International