There are demands on land to provide a variety of ecosystem services alongside agricultural products. In the absence of markets, delivery is generally overseen through separate agencies. However, synergies and trade-offs amongst ecosystem services and variation across space lead to different priorities and opportunities in different areas. This creates a complex challenge for governance and implies a need to devolve decision-making. The objective of this paper is to explore the devolution of decision-making through the introduction of Local Environmental Governance Organisations (LEGO). A LEGO would assemble evidence on natural capital and coordinate stakeholders to identify local priorities. It would search for synergies and collaborative partnerships and raise funds to support priority actions. The paper first sets out a theoretical framework to identify the elements required for local governance. It then proposes two alternatives: a ‘national park’ approach for areas of higher environmental quality and a ‘local nature partnership’ approach elsewhere. The paper then provides a case study of Natural Cambridgeshire, a local nature partnership in England, as a potential LEGO, assessing the extent to which it meets the requirements identified. It has already done much to develop a stakeholder community and has begun to establish priorities for nature enhancement. However, it lacks programmes and long term funding that can incentivise the necessary actions or a forum that can bring together partners for Nature-based Solutions at scale. Central government would need to establish a framework for the operation of a system of LEGOs. It would also continue to support national standards.