The 2022 solar fuels roadmap

dc.contributor.authorSegev, Gideon
dc.contributor.authorKibsgaard, Jakob
dc.contributor.authorHahn, Christopher
dc.contributor.authorXu, Zhichuan J
dc.contributor.authorCheng, Wen-Hui (Sophia)
dc.contributor.authorDeutsch, Todd G
dc.contributor.authorXiang, Chengxiang
dc.contributor.authorZhang, Jenny Z
dc.contributor.authorHammarström, Leif
dc.contributor.authorNocera, Daniel G
dc.contributor.authorWeber, Adam Z
dc.contributor.authorAgbo, Peter
dc.contributor.authorHisatomi, Takashi
dc.contributor.authorOsterloh, Frank E
dc.contributor.authorDomen, Kazunari
dc.contributor.authorAbdi, Fatwa F
dc.contributor.authorHaussener, Sophia
dc.contributor.authorMiller, Daniel J
dc.contributor.authorArdo, Shane
dc.contributor.authorMcIntyre, Paul C
dc.contributor.authorHannappel, Thomas
dc.contributor.authorHu, Shu
dc.contributor.authorAtwater, Harry
dc.contributor.authorGregoire, John M
dc.contributor.authorErtem, Mehmed Z
dc.contributor.authorSharp, Ian D
dc.contributor.authorChoi, Kyoung-Shin
dc.contributor.authorLee, Jae Sung
dc.contributor.authorIshitani, Osamu
dc.contributor.authorAger, Joel W
dc.contributor.authorPrabhakar, Rajiv Ramanujam
dc.contributor.authorBell, Alexis T
dc.contributor.authorBoettcher, Shannon W
dc.contributor.authorVincent, Kylie
dc.contributor.authorTakanabe, Kazuhiro
dc.contributor.authorArtero, Vincent
dc.contributor.authorNapier, Ryan
dc.contributor.authorCuenya, Beatriz Roldan
dc.contributor.authorKoper, Marc T M
dc.contributor.authorVan De Krol, Roel
dc.contributor.authorHoule, Frances
dc.contributor.orcidSegev, Gideon [0000-0002-6175-3458]
dc.contributor.orcidKibsgaard, Jakob [0000-0002-9219-816X]
dc.contributor.orcidHahn, Christopher [0000-0002-2772-6341]
dc.contributor.orcidXu, Zhichuan J [0000-0001-7746-5920]
dc.contributor.orcidCheng, Wen-Hui (Sophia) [0000-0003-3233-4606]
dc.contributor.orcidDeutsch, Todd G [0000-0001-6577-1226]
dc.contributor.orcidZhang, Jenny Z [0000-0003-4407-5621]
dc.contributor.orcidHammarström, Leif [0000-0002-9933-9084]
dc.contributor.orcidNocera, Daniel G [0000-0001-5055-320X]
dc.contributor.orcidWeber, Adam Z [0000-0002-7749-1624]
dc.contributor.orcidAgbo, Peter [0000-0003-3066-4791]
dc.contributor.orcidHisatomi, Takashi [0000-0002-5009-2383]
dc.contributor.orcidOsterloh, Frank E [0000-0002-9288-3407]
dc.contributor.orcidDomen, Kazunari [0000-0001-7995-4832]
dc.contributor.orcidAbdi, Fatwa F [0000-0001-5631-0620]
dc.contributor.orcidHaussener, Sophia [0000-0002-3044-1662]
dc.contributor.orcidArdo, Shane [0000-0001-7162-6826]
dc.contributor.orcidMcIntyre, Paul C [0000-0002-7498-831X]
dc.contributor.orcidHannappel, Thomas [0000-0002-6307-9831]
dc.contributor.orcidHu, Shu [0000-0002-5041-0169]
dc.contributor.orcidAtwater, Harry [0000-0001-9435-0201]
dc.contributor.orcidGregoire, John M [0000-0002-2863-5265]
dc.contributor.orcidErtem, Mehmed Z [0000-0003-1994-9024]
dc.contributor.orcidSharp, Ian D [0000-0001-5238-7487]
dc.contributor.orcidChoi, Kyoung-Shin [0000-0003-1945-8794]
dc.contributor.orcidIshitani, Osamu [0000-0001-9557-7854]
dc.contributor.orcidAger, Joel W [0000-0001-9334-9751]
dc.contributor.orcidBell, Alexis T [0000-0002-5738-4645]
dc.contributor.orcidBoettcher, Shannon W [0000-0001-8971-9123]
dc.contributor.orcidVincent, Kylie [0000-0001-6444-9382]
dc.contributor.orcidTakanabe, Kazuhiro [0000-0001-5374-9451]
dc.contributor.orcidArtero, Vincent [0000-0002-6148-8471]
dc.contributor.orcidNapier, Ryan [0000-0003-1602-7825]
dc.contributor.orcidCuenya, Beatriz Roldan [0000-0002-8025-307X]
dc.contributor.orcidKoper, Marc T M [0000-0001-6777-4594]
dc.contributor.orcidVan De Krol, Roel [0000-0003-4399-399X]
dc.contributor.orcidHoule, Frances [0000-0001-5571-2548]
dc.date.accessioned2022-06-29T19:44:04Z
dc.date.available2022-06-29T19:44:04Z
dc.date.issued2022-06-22
dc.date.submitted2021-11-05
dc.date.updated2022-06-29T19:44:03Z
dc.descriptionFunder: Alfred P. Sloan Foundation; doi: http://dx.doi.org/10.13039/100000879
dc.descriptionFunder: Thistledown Foundation
dc.descriptionFunder: Research Corporation for Science Advancement; doi: http://dx.doi.org/10.13039/100001309
dc.descriptionFunder: TomKat Foundation; doi: http://dx.doi.org/10.13039/100018042
dc.descriptionFunder: Taiwan Ministry of Education and Taiwan and Ministry of Science
dc.descriptionFunder: the Netherlands Ministry of Economic Affairs and Climate Policy
dc.descriptionFunder: Nederlandse Organisatie voor Wetenschappelijk Onderzoek; doi: http://dx.doi.org/10.13039/501100003246
dc.description.abstractAbstract: Renewable fuel generation is essential for a low carbon footprint economy. Thus, over the last five decades, a significant effort has been dedicated towards increasing the performance of solar fuels generating devices. Specifically, the solar to hydrogen efficiency of photoelectrochemical cells has progressed steadily towards its fundamental limit, and the faradaic efficiency towards valuable products in CO2 reduction systems has increased dramatically. However, there are still numerous scientific and engineering challenges that must be overcame in order to turn solar fuels into a viable technology. At the electrode and device level, the conversion efficiency, stability and products selectivity must be increased significantly. Meanwhile, these performance metrics must be maintained when scaling up devices and systems while maintaining an acceptable cost and carbon footprint. This roadmap surveys different aspects of this endeavor: system benchmarking, device scaling, various approaches for photoelectrodes design, materials discovery, and catalysis. Each of the sections in the roadmap focuses on a single topic, discussing the state of the art, the key challenges and advancements required to meet them. The roadmap can be used as a guide for researchers and funding agencies highlighting the most pressing needs of the field.
dc.identifier.doi10.17863/CAM.85882
dc.identifier.eissn1361-6463
dc.identifier.issn0022-3727
dc.identifier.otherdac6f97
dc.identifier.otherac6f97
dc.identifier.otherjphysd-129688.r1
dc.identifier.urihttps://www.repository.cam.ac.uk/handle/1810/338469
dc.languageen
dc.publisherIOP Publishing
dc.subjectRoadmap
dc.subjectsolar fuels
dc.subjectcatalysis
dc.subjectCO2 reduction
dc.subjectwater splitting
dc.titleThe 2022 solar fuels roadmap
dc.typeArticle
dcterms.dateAccepted2022-05-13
prism.issueIdentifier32
prism.publicationNameJournal of Physics D: Applied Physics
prism.volume55
pubs.funder-project-idKorean Ministry of Science (NRF-2018R1A2A1A05077909, NRF-2019M1A2A2065612)
pubs.funder-project-idU.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Fuels from Sunlight Hub (DE-SC0021266)
pubs.funder-project-idHorizon 2020 Framework Programme (864234, 883264)
pubs.funder-project-idNational Science Foundation (CBET-1805084)
pubs.funder-project-idSchweizerischer Nationalfonds zur Förderung der Wissenschaftlichen Forschung (155876, 191299)
pubs.funder-project-idBiotechnology and Biological Sciences Research Council (BB/R011923/1, BB/R018413/1)
pubs.funder-project-idU.S. Department of Energy (DE-AC36-08GO28308, DE-EE0008092, DE-SC0004993, DE-SC0008707, DE-SC0017619, DE-SC0021173, DE-SC0021266, DE-SC0021953, DE-SC00493)
pubs.funder-project-idLawrence Livermore National Laboratory (19-SI-005, DE-AC52-07NA27344)
pubs.funder-project-idAgence Nationale de la Recherche (Labex ARCANE, CBH-EUR-GS, ANR-17-EURE-0003, BEEP)
pubs.funder-project-idEuropean Research Council (ERC-2018-CoG BiocatSusChem 819580)
pubs.funder-project-idCarlsbergfondet (CF18-0435)
pubs.funder-project-idMohammed bin Salman Center (MbSC2030)
pubs.funder-project-idDeutsche Forschungsgemeinschaft (3096/10, 3096/19, 406944504 – SPP 2080, 981)
pubs.funder-project-idJapan Society for the Promotion of Science (JP17H06440, JP20H00396)
pubs.funder-project-idGerman Federal Ministry of Education and Research (033RC021A, 033RC021C, 03SF0619C, 03SF0619I)
pubs.funder-project-idNSF Chemical Catalysis (1955106)
rioxxterms.licenseref.urihttp://creativecommons.org/licenses/by/4.0
rioxxterms.versionVoR
rioxxterms.versionofrecord10.1088/1361-6463/ac6f97
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