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dc.contributor.authorXomalis, Angelos
dc.contributor.authorZheng, Xuezhi
dc.contributor.authorChikkaraddy, Rohit
dc.contributor.authorKoczor-Benda, Zsuzsanna
dc.contributor.authorMiele, Ermanno
dc.contributor.authorRosta, Edina
dc.contributor.authorVandenbosch, Guy AE
dc.contributor.authorMartínez, Alejandro
dc.contributor.authorBaumberg, Jeremy
dc.date.accessioned2021-11-17T00:31:15Z
dc.date.available2021-11-17T00:31:15Z
dc.date.issued2021-12-03
dc.identifier.issn0036-8075
dc.identifier.urihttps://www.repository.cam.ac.uk/handle/1810/330701
dc.description.abstract<jats:title>Optomechanical upconversion</jats:title> <jats:p> Molecules have rich signatures in their spectra at infrared wavelengths and are typically accessed with dedicated spectroscopic instrumentation. Chen <jats:italic>et al</jats:italic> . and Xomalis <jats:italic>et al</jats:italic> . report optomechanical frequency upconversion from the mid-infrared to the visible domain using molecular vibrations coupled to a plasmonic nanocavity at ambient conditions (see the Perspective by Gordon). Using different nanoantenna designs, one with a nanoparticle-on-resonator and the other with nanoparticle-in-groove, both approaches show the ability to upconvert the mid-infrared vibrations of the molecules in the nanocavity to visible light wavelengths. The effect could be used to simplify infrared spectroscopy, possibly with single-molecule sensitivity. —ISO </jats:p>
dc.publisherAmerican Association for the Advancement of Science (AAAS)
dc.rightsAll rights reserved
dc.rights.urihttp://www.rioxx.net/licenses/all-rights-reserved
dc.titleDetecting mid-infrared light by molecular frequency upconversion in dual-wavelength nanoantennas
dc.typeArticle
prism.publicationNameScience
dc.identifier.doi10.17863/CAM.78146
dcterms.dateAccepted2021-10-12
rioxxterms.versionofrecord10.1126/science.abk2593
rioxxterms.versionAM
rioxxterms.licenseref.urihttp://www.rioxx.net/licenses/all-rights-reserved
rioxxterms.licenseref.startdate2021-10-12
dc.contributor.orcidXomalis, Angelos [0000-0001-8406-9571]
dc.contributor.orcidChikkaraddy, Rohit [0000-0002-3840-4188]
dc.contributor.orcidKoczor-Benda, Zsuzsanna [0000-0002-6714-0337]
dc.contributor.orcidMiele, Ermanno [0000-0001-5085-9815]
dc.contributor.orcidMartínez, Alejandro [0000-0001-5448-0140]
dc.contributor.orcidBaumberg, Jeremy [0000-0002-9606-9488]
dc.identifier.eissn1095-9203
rioxxterms.typeJournal Article/Review
pubs.funder-project-idEngineering and Physical Sciences Research Council (EP/L027151/1)
pubs.funder-project-idEuropean Commission Horizon 2020 (H2020) Future and Emerging Technologies (FET) (829067)
pubs.funder-project-idEuropean Commission Horizon 2020 (H2020) Research Infrastructures (RI) (861950)
pubs.funder-project-idEuropean Commission Horizon 2020 (H2020) ERC (883703)
datacite.issupplementedby.urlhttps://doi.org/10.17863/CAM.77640
cam.orpheus.successTue Feb 01 19:02:17 GMT 2022 - Embargo updated*
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rioxxterms.freetoread.startdate2021-12-03


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