Zip folder containing .txt files of steady-state spectroscopy data. The TA folder contains .txt files of the TA spectra for polycrystalline thin films. The XRD folder contains .txt files for experimental and simulated XRD patterns. The TAM folder contains .txt files for the kinetics, fitted parameters and fluence dependence for fitted parameters. The computational folder contains JPEG and pdf files for high-quality band structures, orbital plots and crystal structures.