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dc.contributor.authorWirnsberger, Peteren
dc.contributor.authorFijan, Den
dc.contributor.authorLightwood, RAen
dc.contributor.authorŠarić, Aen
dc.contributor.authorDellago, Cen
dc.contributor.authorFrenkel, Daanen
dc.date.accessioned2017-06-05T11:08:11Z
dc.date.available2017-06-05T11:08:11Z
dc.date.issued2017-05-09en
dc.identifier.issn0027-8424
dc.identifier.urihttps://www.repository.cam.ac.uk/handle/1810/264628
dc.description.abstractElectric charges are conserved. The same would be expected to hold for magnetic charges, yet magnetic monopoles have never been observed. It is therefore surprising that the laws of nonequilibrium thermodynamics, combined with Maxwell's equations, suggest that colloidal particles heated or cooled in certain polar or paramagnetic solvents may behave as if they carry an electric/magnetic charge. Here, we present numerical simulations that show that the field distribution around a pair of such heated/cooled colloidal particles agrees quantitatively with the theoretical predictions for a pair of oppositely charged electric or magnetic monopoles. However, in other respects, the nonequilibrium colloidal particles do not behave as monopoles: They cannot be moved by a homogeneous applied field. The numerical evidence for the monopole-like fields around heated/cooled colloidal particles is crucial because the experimental and numerical determination of forces between such colloidal particles would be complicated by the presence of other effects, such as thermophoresis.
dc.description.sponsorshipWe acknowledge financial support from the Austrian Academy of Sciences through a doctoral (DOC) fellowship (to P.W.), the Austrian Science Fund (FWF) within the Spezialforschungsbereich Vienna Computational Materials Laboratory (Project F41) (C.D.), and the European Union Early Training Network NANOTRANS (Grant 674979 to D. Frenkel). The results presented here have been achieved in part using the Vienna Scientific Cluster.
dc.languageengen
dc.language.isoenen
dc.publisherNational Academy of Sciences
dc.subjectcolloidsen
dc.subjectmolecular simulationen
dc.subjectmonopolesen
dc.subjectnonequilibrium thermodynamicsen
dc.subjectsoft matteren
dc.titleNumerical evidence for thermally induced monopolesen
dc.typeArticle
prism.endingPage4914
prism.issueIdentifier19en
prism.publicationDate2017en
prism.publicationNameProceedings of the National Academy of Sciences of the United States of Americaen
prism.startingPage4911
prism.volume114en
dc.identifier.doi10.17863/CAM.10211
dcterms.dateAccepted2017-03-16en
rioxxterms.versionofrecord10.1073/pnas.1621494114en
rioxxterms.versionAMen
rioxxterms.licenseref.urihttp://www.rioxx.net/licenses/all-rights-reserveden
rioxxterms.licenseref.startdate2017-05-09en
dc.contributor.orcidWirnsberger, Peter [0000-0001-5961-5817]
dc.contributor.orcidFrenkel, Daan [0000-0002-6362-2021]
dc.identifier.eissn1091-6490
rioxxterms.typeJournal Article/Reviewen
pubs.funder-project-idEuropean Commission Horizon 2020 (H2020) Marie Sk?odowska-Curie actions (674979)
cam.issuedOnline2017-04-24en
datacite.issupplementedby.doi10.17863/CAM.8607en
rioxxterms.freetoread.startdate2017-10-24


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