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Electrically tunable stacking domains and ferroelectricity in moiré superlattices

cam.depositDate2021-12-03
cam.orpheus.counter6*
cam.orpheus.success2022-05-17
dc.contributor.authorBennett, Daniel
dc.contributor.authorRemez, Benjamin
dc.contributor.orcidBennett, Daniel [0000-0003-0892-2125]
dc.date.accessioned2021-12-09T00:30:12Z
dc.date.available2021-12-09T00:30:12Z
dc.date.updated2021-12-03T13:28:09Z
dc.description.abstractIt is well known that stacking domains form in moir\'e superlattices due to the competition between the interlayer van der Waals forces and intralayer elastic forces, which can be recognized as polar domains due to the local spontaneous polarization in bilayers without centrosymmetry. We propose a theoretical model which captures the effect of an applied electric field on the domain structure. The coupling between the spontaneous polarization and field leads to uneven relaxation of the domains, and a net polarization in the superlattice at nonzero fields, which is sensitive to the moir\'e period. We show that the dielectric response to the field reduces the stacking energy and leads to softer domains in all bilayers. We then discuss the recent observations of ferroelectricity in the context of our model.
dc.identifier.doi10.17863/CAM.78721
dc.identifier.urihttps://www.repository.cam.ac.uk/handle/1810/331274
dc.language.isoeng
dc.publisher.departmentDepartment of Physics Student
dc.rightsCreative Commons CC BY 4.0
dc.rights.urihttp://www.rioxx.net/licenses/CC BY 4.0
dc.subjectcond-mat.mes-hall
dc.subjectcond-mat.mes-hall
dc.titleElectrically tunable stacking domains and ferroelectricity in moiré superlattices
dc.typeArticle
pubs.licence-display-nameApollo Repository Deposit Licence Agreement
pubs.licence-identifierapollo-deposit-licence-2-1
rioxxterms.typeJournal Article/Review
rioxxterms.versionVoR

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