Room temperature polaritonic soft-spin XY Hamiltonian in organic-inorganic halide perovskites
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Peer-reviewed
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jats:titleAbstract</jats:title> jats:pExciton–polariton condensates, due to their nonlinear and coherent characteristics, have been employed to construct spin Hamiltonian lattices for potentially studying spin glass, critical dephasing, and even solving optimization problems. Here, we report the room-temperature polariton condensation and polaritonic soft-spin XY Hamiltonian lattices in an organic–inorganic halide perovskite microcavity. This is achieved through the direct integration of high-quality single-crystal samples within the cavity. The ferromagnetic and antiferromagnetic couplings in both one- and two-dimensional condensate lattices have been observed clearly. Our work shows a nonlinear organic–inorganic hybrid perovskite platform for future investigations as polariton simulators.</jats:p>
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Peer reviewed: True
Acknowledgements: We thank A. Gao from SVOTEK Inc. for assisting with the high-quality DBR mirror coating.
Publication status: Published
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2192-8614
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Office of Naval Research (N00014-21-1-2099, N00014-22-1-2322)
National Science Foundation (DMR-2414131)
Julian Schwinger Foundation for Physics Research (JSF-19-02-0005)
Weizmann-UK grant (142568)
HORIZON EUROPE (UKRI G123670)