This includes the FIDs and processed spectra of all NMR experiments published in the paper "NMR Reveals the Surface Functionalisation of Ti3C2 MXene". Specifically, this is 1H, 13C and 19F NMR experiments as well as 1H-13C and 1H-19F correlation experiments for Ti3C2 MXene. Please see the paper for more details. The files are provided in the JCAMP-DX format, for which there are non-proprietary software packages available. However, these files were generated by Bruker's TopSpin, and time domain data in particular may only load correctly using this program. The pulse sequences used are also provided in the TopSpin format.