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Terahertz saturable absorbers from liquid phase exfoliation of graphite

Published version
Peer-reviewed

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Authors

Bianchi, V 
Carey, T 
Viti, L 
Li, L 
Linfield, EH 

Abstract

Saturable absorbers (SA) operating at terahertz (THz) frequencies can open new frontiers in the development of passively mode-locked THz micro-sources. Here we report the fabrication of THz SAs by transfer coating and inkjet printing single and few-layer graphene films prepared by liquid phase exfoliation of graphite. Open-aperture z-scan measurements with a 3.5 THz quantum cascade laser show a transparency modulation ∼80%, almost one order of magnitude larger than that reported to date at THz frequencies. Fourier-transform infrared spectroscopy provides evidence of intraband-controlled absorption bleaching. These results pave the way to the integration of graphene-based SA with electrically pumped THz semiconductor micro-sources, with prospects for applications where excitation of specific transitions on short time scales is essential, such as time-of-flight tomography, coherent manipulation of quantum systems, time-resolved spectroscopy of gases, complex molecules and cold samples and ultra-high speed communications, providing unprecedented compactness and resolution.

Description

Keywords

0202 Atomic, Molecular, Nuclear, Particle and Plasma Physics, 0205 Optical Physics

Journal Title

Nature Communications

Conference Name

Journal ISSN

2041-1723
2041-1723

Volume Title

8

Publisher

Nature Publishing Group
Sponsorship
Engineering and Physical Sciences Research Council (EP/G042357/1)
The Royal Society (wm090070)
Isaac Newton Trust (1135(N))
Engineering and Physical Sciences Research Council (EP/K017144/1)
Engineering and Physical Sciences Research Council (EP/J017671/1)
Engineering and Physical Sciences Research Council (EP/K01711X/1)
Engineering and Physical Sciences Research Council (EP/L016087/1)
Engineering and Physical Sciences Research Council (EP/P02534X/1)
Engineering and Physical Sciences Research Council (EP/N010345/1)
We acknowledge funding from ERC grants SPRINT, Hetero2D, HiGRAPHINK, the EU Graphene Flagship, and EPSRC grants EP/K01711X/1, EP/K017144/1, EP/L016087/1 and EP/N010345/1.