Structural modulation and assembling of metal halide perovskites for solar cells and light-emitting diodes
Publication Date
2021Journal Title
INFOMAT
ISSN
2567-3165
Publisher
Wiley
Volume
3
Issue
11
Pages
1218-1250
Language
en
Type
Article
This Version
AO
VoR
Metadata
Show full item recordCitation
Liu, X., Zhang, Z., Lin, F., & Cheng, Y. (2021). Structural modulation and assembling of metal halide perovskites for solar cells and light-emitting diodes. INFOMAT, 3 (11), 1218-1250. https://doi.org/10.1002/inf2.12256
Description
Funder: Singapore Economic Development Board
Funder: Energy Market Authority of Singapore; Id: http://dx.doi.org/10.13039/501100001447
Funder: National Research Foundation Singapore; Id: http://dx.doi.org/10.13039/501100001381
Funder: National University of Singapore; Id: http://dx.doi.org/10.13039/501100001352
Funder: International Postdoctoral Exchange Fellowship Program (Talent‐Introduction Program) of China
Funder: Boya Postdoctoral program of Peking University
Abstract
Abstract: Metal halide perovskites possess appealing optoelectronic properties and have been widely applied for solar energy harvesting and light emitting. Although perovskite solar cells (PeSCs) and perovskite light‐emitting diodes (PeLEDs) have been developed rapidly in recent years, there are still no universal rules for the selection of perovskites to achieve high‐performance optoelectronic devices. In this review, the working mechanisms of PeSCs and PeLEDs are first demonstrated with the discussion on the factors which determine the device performance. We then examine the optoelectronic properties of perovskites with structures modulated from 3D, 2D, 1D to 0D, and analyze the corresponding structure‐property relationships in terms of photo‐electric and electric‐photo conversion processes. Based on the unique optoelectronic properties of structurally modulated perovskites, we put forward the concept of structural assembling engineering that integrate the merits of different types of perovskites within one matrix and elaborate their excellent properties for applications of both PeSCs and PeLEDs. Finally, we discuss the potential challenges and provide our perspectives on the structural assembling engineering of perovskites for future optoelectronic applications. image
Keywords
REVIEW ARTICLE, REVIEW ARTICLES, light‐emitting diodes, low‐dimensional perovskites, metal halide perovskites, solar cells, structural assembling, structure modulation
Identifiers
inf212256
External DOI: https://doi.org/10.1002/inf2.12256
This record's URL: https://www.repository.cam.ac.uk/handle/1810/330838
Rights
Licence:
http://creativecommons.org/licenses/by/4.0/
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