Very High Surface Area Mesoporous Thin Films of SrTiO$_{3}$  Grown by Pulsed Laser Deposition and Application to Efficient Photoelectrochemical Water Splitting

Sangle, AL; Singh, S; Jian, J; Bajpe, SR; Wang, H; Khare, N; MacManus-Driscoll, JL

Very High Surface Area Mesoporous Thin Films of SrTiO$_{3}$ Grown by Pulsed Laser Deposition and Application to Efficient Photoelectrochemical Water Splitting

Accepted version

Peer-reviewed

Repository URI

https://www.repository.cam.ac.uk/handle/1810/261845

Repository DOI

https://doi.org/10.17863/CAM.7065

Files

Accepted version (647.17 KB)

Type

Article

Authors

Sangle, AL

Singh, S

Jian, J

Bajpe, SR

Wang, H

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Abstract

Very high surface area, self-assembled, highly crystalline mesoporous SrTiO $3$ (STO) thin films were developed for photoelectrochemical water splitting. Much improved performance of these mesoporous films compared to planar STO thin films and any other form of STO such as single crystal samples and nanostructures was demonstrated. The high performance resulted from very large surface area films and optimization of carrier concentration.

Keywords

high surface area films, mesoporous crystalline thin films, photoelectrochemical water splitting, pulsed laser deposition, self-assembled nanocomposite films, SrTiO$_{3}$

Journal Title

Nano Letters

Journal ISSN

1530-6984
1530-6992

Volume Title

16

Publisher

American Chemical Society

Publisher DOI

https://doi.org/10.1021/acs.nanolett.6b02487

Rights

http://www.rioxx.net/licenses/all-rights-reserved

Sponsorship

European Research Council (247276)

We gratefully acknowledge the support from the Cambridge Commonwealth Trust, ERC adg grant (247276) NOVOX and UKIERI grant (IND/CONT/E/12-13/813). The TEM work at Texas A&M University is funded by the US National Science Foundation (DMR-1401266).

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Scholarly Works - Materials Science and Metallurgy
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